A method for removing atmospheric carbon dioxide (СО2) and water vapor is proposed. The method sprays clouds with alkaline compounds to significantly increase the solubility of СО2 in the cloud water, providing for much higher than normal levels of СО2 to be absorbed by rain droplets. The CO2 is transported to the ground for sequestration in surface and/or ground water, and available for carbon fixation by plants and organisms. Presented calculations estimate that 38 gigatonnes of atmospheric CO2 could be removed per year by applying the process over 0.08% to 2.4 % of the Earth’s surface. Laboratory experiments that grew multiple edible plant species irrigated with the modified rainwater indicated yield benefits. A concept for removing atmospheric methane (CH4) is also presented. Powerful lasers would ionize the CH4 to form CO2 that could then be removed by the alkaline-enhanced rainfall method.
Published in |
American Journal of Environmental Protection (Volume 5, Issue 3-1)
This article belongs to the Special Issue New Technologies and Geoengineering Approaches for Climate |
DOI | 10.11648/j.ajep.s.2016050301.14 |
Page(s) | 21-25 |
Creative Commons |
This is an Open Access article, distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution and reproduction in any medium or format, provided the original work is properly cited. |
Copyright |
Copyright © The Author(s), 2016. Published by Science Publishing Group |
Climate Change, Greenhouse Gas, Carbon Dioxide, Methane, Water Vapor, Removal, Alkali, pH Adjustment, Precipitation, Cloud Seeding, Laser
[1] | IPCC, Contribution of Working Group III to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change. Summary for Policymakers, Cambridge University Press, New York, 2014. |
[2] | Kleidon, A., Malhi, Y. and Cox, P. M., “Maximum entropy production in environmental and ecological systems introduction,” Philos. Trans. R. Soc. B 365, 1297-1302. 2010. |
[3] | Freidenreich, S. M. and Ramaswamy, V., “Solar radiation absorption by carbon dioxide, overlap with water, and a parameterization for general circulation models,” J. of Geophys. Res. 98, 7255-7264. 1993. |
[4] | Latest reading, Mauna Loa Observatory. 2016. https://scripps.ucsd.edu/programs/keelingcurve/. [Accessed Apr. 4, 2016]. |
[5] | Schmidt, G., “Methane: a scientific journey from obscurity to climate super-stardom,” NASA Goddard Space Center, 2004. http://www.giss.nasa.gov/research/features/200409_methane/.[Accessed Apr. 4, 2016]. |
[6] | Andersson, A. J. and Gledhill, D., “Ocean acidification and coral reefs: effects on breakdown, dissolution, and net ecosystem calcification,” Annu Rev Mar Sci 5, 1.1–1.28, 2013. |
[7] | Secretariat of the Convention on Biological Diversity, Roberts, J. M. and Williamson, P. – ed., An Updated Synthesis of the Impacts of Ocean Acidification on Marine Biodiversity, Technical Series No. 75, Montreal, Canada, 2014. |
[8] | Izrael, Y. A. et al., Acid rain (Hydrometeoisdat, Russia, 1989). |
[9] | Langmuir, I., “Improved methods of conditioning surfaces for adsorption” J. Am. Chem. Soc. 59. 1762-1763. 1937. |
[10] | Dennis, A. S., Weather modification by cloud seeding, Academic Press, New York, 1980. |
[11] | Shmeter, S. M. and Berynlev, G. P., “Efficiency of cloud and precipitation modification with hygroscopic aerosols,” Meteorology and Hydrology Rus., 2. 43-60. 2005. |
[12] | Tulaikova, T., Mihtchenko, A. and Amirova, S., “Micro physical model for glaciogenic particles in clouds for precipitation enhancement,” Am. J. Env. Protection, 5(3-1). 10-14. 2016. |
[13] | Tulaikova, T. et al., Acoustic rains, Physmathbook, Moscow, 2010. |
[14] | Claus R. O. and Tulaikova, T. V., “New methods for helicopter for free flight inside clouds and precipitation enhancement,” Am. J. Env. Protection, 5. 1-9. 2016. |
[15] | Yunge, H., Chemical compounds and radio-activity in the atmosphere, Clarendon, Oxford, 1965. |
[16] | Rasool, S. I. (ed.), Chemistry of the lower atmosphere, Plenum, New York, 1973. |
[17] | Sillen, L. G. (ed.), Stability constants of metal-ion complexes, Chemical Society, London, 1964. |
[18] | Borovikov, A. M., Physics of clouds, Hydromet-Press, Leningrad, Russia, 1961. |
[19] | Kobayashi, S. T. et al, “Backscattering enhancement on spheroid-shaped hydrometeors: considerations in water and ice particles of uniform size and Marshall-Palmer distributed rains,” Radio Science, 42. Apr.2007. |
[20] | Bruintjes, R. T., “A review of cloud seeding experiments to enhance precipitation and some new prospects,” BAMS, 90. 805-820. 1999. |
[21] | Daly, C. et al, “Observation bias in daily precipitation measurements at United States cooperative network stations,” BAMS 88. 899-912. 2007. |
[22] | Taylor, J. W. et al, “Aerosol measurements during COPE: composition, size and sources of CCN and IN at the interface between marine and terrestrial influences,” Atmos. Chem. Phys. Discuss., doi: 10.5194/acp-2016-84, in review. 2016. |
[23] | Hoover, T. E., “CO2 exchange at the air-sea interface,” J. Geoph.Res 74. 456-464. 1969. |
[24] | Liss, P. S., “Processes of gas exchange analysis an air-water interface,” Deep-Sea Res. 20. 221-238. 1973. |
[25] | Broecher, H. C., “The influence of wind on CO2 exchange in a wind-water tunnel including the effect of minelayers,” J. Mar. Res. 36. 595-610. 1978. |
[26] | Wanninkhof, R., “Chemical enhancement of CO2 exchange in natural water,” Limnol. Oceanogr., 41. 689-687. 1996. |
[27] | Tulaikova, T., and Amirova, S., “The method for effective CO2 purification in the atmosphere,” Global J. Sc. Frontier Res., 15-H (1). 1-9. 2015. |
[28] | Rees, G. and Rees, W., Physical principles of remote sensing, Cambridge University Press, 2013, 125. |
[29] | Olivier, J., Janssens-Maenhout, G., Muntean, M. and Peters, J., Trends in global CO2 emissions: 2015 report, PBL Netherlands Environmental Assessment Agency, 2015. |
[30] | Food and Agriculture Organization of the United Nations, “World fertilizer trends and outlook to 2018,” Rome, Italy, 2015. |
[31] | Sheu, J., Mokheimer, E. and Ghoniem, A., “A review of solar methane reforming systems,” Int. J. Hydrogen Energy, 40. 12929-12955. 2015. |
[32] | Clark, J., Calculations in AS/A Level Chemistry, Pearson Education, London, 2000. |
[33] | Dawsey, M. et al, “Optical parametric technology for methane measurements,” Proc. 2015 SPIE, Lidar Remote Sensing for Environmental Monitoring XV, San Diego, USA. |
[34] | Riris, H. et al, “Airborne measurements of atmospheric methane column abundance using a pulsed integrated-path differential absorption Lidar,” Applied Optics, 51 (34). 8296- 8305. 2012. |
[35] | Schmidt, W., Optical spectroscopy in chemistry and life sciences, Wiley-VCH, Germany, 2005. |
[36] | Cantrell, C. D. (ed.), Multiple-photon excitation and dissociation of polyatomic molecules, Springer, New York, 1986. |
[37] | Brien, J. and Cao, H., “Absorption spectra and absorption coefficients for methane in the 750–940 nm region obtained by intracavity laser spectroscopy,” J. Quant. Spec. Rad. Tran., 75 (3). 323-350. Oct. 2002. |
APA Style
John B. Cook, Svetlana R. Amirova, Edwin A. Roehl Jr., Paul A. Comet, Tamara V. Tulaykova. (2016). An Approach to Removing Large Quantities of Atmospheric Greenhouse Gases. American Journal of Environmental Protection, 5(3-1), 21-25. https://doi.org/10.11648/j.ajep.s.2016050301.14
ACS Style
John B. Cook; Svetlana R. Amirova; Edwin A. Roehl Jr.; Paul A. Comet; Tamara V. Tulaykova. An Approach to Removing Large Quantities of Atmospheric Greenhouse Gases. Am. J. Environ. Prot. 2016, 5(3-1), 21-25. doi: 10.11648/j.ajep.s.2016050301.14
AMA Style
John B. Cook, Svetlana R. Amirova, Edwin A. Roehl Jr., Paul A. Comet, Tamara V. Tulaykova. An Approach to Removing Large Quantities of Atmospheric Greenhouse Gases. Am J Environ Prot. 2016;5(3-1):21-25. doi: 10.11648/j.ajep.s.2016050301.14
@article{10.11648/j.ajep.s.2016050301.14, author = {John B. Cook and Svetlana R. Amirova and Edwin A. Roehl Jr. and Paul A. Comet and Tamara V. Tulaykova}, title = {An Approach to Removing Large Quantities of Atmospheric Greenhouse Gases}, journal = {American Journal of Environmental Protection}, volume = {5}, number = {3-1}, pages = {21-25}, doi = {10.11648/j.ajep.s.2016050301.14}, url = {https://doi.org/10.11648/j.ajep.s.2016050301.14}, eprint = {https://article.sciencepublishinggroup.com/pdf/10.11648.j.ajep.s.2016050301.14}, abstract = {A method for removing atmospheric carbon dioxide (СО2) and water vapor is proposed. The method sprays clouds with alkaline compounds to significantly increase the solubility of СО2 in the cloud water, providing for much higher than normal levels of СО2 to be absorbed by rain droplets. The CO2 is transported to the ground for sequestration in surface and/or ground water, and available for carbon fixation by plants and organisms. Presented calculations estimate that 38 gigatonnes of atmospheric CO2 could be removed per year by applying the process over 0.08% to 2.4 % of the Earth’s surface. Laboratory experiments that grew multiple edible plant species irrigated with the modified rainwater indicated yield benefits. A concept for removing atmospheric methane (CH4) is also presented. Powerful lasers would ionize the CH4 to form CO2 that could then be removed by the alkaline-enhanced rainfall method.}, year = {2016} }
TY - JOUR T1 - An Approach to Removing Large Quantities of Atmospheric Greenhouse Gases AU - John B. Cook AU - Svetlana R. Amirova AU - Edwin A. Roehl Jr. AU - Paul A. Comet AU - Tamara V. Tulaykova Y1 - 2016/05/10 PY - 2016 N1 - https://doi.org/10.11648/j.ajep.s.2016050301.14 DO - 10.11648/j.ajep.s.2016050301.14 T2 - American Journal of Environmental Protection JF - American Journal of Environmental Protection JO - American Journal of Environmental Protection SP - 21 EP - 25 PB - Science Publishing Group SN - 2328-5699 UR - https://doi.org/10.11648/j.ajep.s.2016050301.14 AB - A method for removing atmospheric carbon dioxide (СО2) and water vapor is proposed. The method sprays clouds with alkaline compounds to significantly increase the solubility of СО2 in the cloud water, providing for much higher than normal levels of СО2 to be absorbed by rain droplets. The CO2 is transported to the ground for sequestration in surface and/or ground water, and available for carbon fixation by plants and organisms. Presented calculations estimate that 38 gigatonnes of atmospheric CO2 could be removed per year by applying the process over 0.08% to 2.4 % of the Earth’s surface. Laboratory experiments that grew multiple edible plant species irrigated with the modified rainwater indicated yield benefits. A concept for removing atmospheric methane (CH4) is also presented. Powerful lasers would ionize the CH4 to form CO2 that could then be removed by the alkaline-enhanced rainfall method. VL - 5 IS - 3-1 ER -